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Transmission-based charge modulation microscopy on conjugated polymer blend field-effect transistors.

Authors :
Zhang, Yansheng
Nguyen, Malgorzata
Schnedermann, Christoph
Keene, Scott T.
Jacobs, Ian
Rao, Akshay
Sirringhaus, Henning
Source :
Journal of Chemical Physics. 1/21/2023, Vol. 158 Issue 3, p1-8. 8p.
Publication Year :
2023

Abstract

Charge modulation microscopy (CMM) is an electro-optical method that is capable of mapping the spatial distribution of induced charges in an organic field-effect transistor (OFET). Here, we report a new (and simple) implementation of CMM in transmission geometry with camera-based imaging. A significant improvement in data acquisition speed (by at least an order of magnitude) has been achieved while preserving the spatial and spectral resolution. To demonstrate the capability of the system, we measured the spatial distribution of the induced charges in an OFET with a polymer blend of indacenodithiophene-co-benzothiadiazole and poly-vinylcarbazole that shows micrometer-scale phase separation. We were able to resolve spatial variations in the accumulated charge density on a length scale of 500 nm. We demonstrated through a careful spectral analysis that the measured signal is a genuine charge accumulation signal that is not dominated by optical artifacts. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
00219606
Volume :
158
Issue :
3
Database :
Academic Search Index
Journal :
Journal of Chemical Physics
Publication Type :
Academic Journal
Accession number :
161416345
Full Text :
https://doi.org/10.1063/5.0132426