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Shape Anisotropic Chain‐Like CoNi/Polydimethylsiloxane Composite Films with Excellent Low‐Frequency Microwave Absorption and High Thermal Conductivity.
- Source :
-
Advanced Functional Materials . Feb2024, p1. 10p. 7 Illustrations. - Publication Year :
- 2024
-
Abstract
- The demand for low‐frequency microwave absorption materials is becoming more and more urgent. Novel shape anisotropy chain‐like CoNi is fabricated using polyvinylpyrrolidone as a shape‐directing agent via solvothermal method, which is then mixed with polydimethylsiloxane (PDMS) to prepare corresponding multifunctional chain‐like CoNi/PDMS composite films. Shape anisotropy and strong magnetic coupling effect of chain‐like CoNi enhance natural resonance and magnetic loss capability. The minimum reflection loss (RLmin) is −50.5 dB and low‐frequency effective absorption bandwidth (EAB) is 1.04 GHz (2.64–3.68 GHz) at 3.9 mm for chain‐like CoNi. The corresponding 18 vol% chain‐like CoNi/PDMS composite films present optimal low‐frequency microwave absorption performance with RLmin of −56.7 dB and low‐frequency EAB of 1.04 GHz (2.96–4.00 GHz) at 4.1 mm, which is far superior to 18 vol% spherical CoNi/PDMS composite films with RLmin of −9.5 dB. Meantime, the in‐plane and inter‐plane thermal conductivity coefficients of 18 vol% chain‐like CoNi/PDMS composite films are 2.05 and 0.61 W m−1 K−1, about 1.5 times higher than 18 vol% spherical CoNi/PDMS composite films (1.36 and 0.42 W m−1 K−1), also 220% and 190% higher than pure PDMS (0.64 and 0.21 W m−1 K−1). This composite films with low‐frequency microwave absorption and thermal conductivity can broaden applications in 5G communications and flexible electronics. [ABSTRACT FROM AUTHOR]
Details
- Language :
- English
- ISSN :
- 1616301X
- Database :
- Academic Search Index
- Journal :
- Advanced Functional Materials
- Publication Type :
- Academic Journal
- Accession number :
- 175386139
- Full Text :
- https://doi.org/10.1002/adfm.202316691