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Manganese oxide-based catalysts for the sustainable synthesis of value-added chemicals through oxidation processes: a critical review and perspectives for the future.
- Source :
-
Green Chemistry . 3/7/2024, Vol. 26 Issue 5, p2365-2383. 19p. - Publication Year :
- 2024
-
Abstract
- The use of manganese oxide (MnOx)-based catalysts has gained significant recognition as a promising solution for the sustainable synthesis of value-added chemicals. These catalysts possess notable qualities such as exceptional catalytic performance, cost-effectiveness, stability, and environmentally friendly properties. This review provides an overview of three typical processes for constructing novel MnOx-based catalysts through vacancy engineering, facet engineering, and crystal-phase engineering. It then discusses advancements made in the past five years in the sustainable synthesis of value-added chemicals using these MnOx-based heterogeneous catalysts. This includes the aerobic oxidation of alcohols and hydrocarbons, homo/cross-coupling of C–N/N=N bonds, and biomass transformation. The review emphasizes the crucial role played by vacancy engineering, crystal-phase engineering, and facet engineering of MnOx-based heterogeneous catalysts in sustainable chemical synthesis. Lastly, it discusses the general challenges and future directions of this exciting area of research. [ABSTRACT FROM AUTHOR]
Details
- Language :
- English
- ISSN :
- 14639262
- Volume :
- 26
- Issue :
- 5
- Database :
- Academic Search Index
- Journal :
- Green Chemistry
- Publication Type :
- Academic Journal
- Accession number :
- 175824706
- Full Text :
- https://doi.org/10.1039/d3gc04117d