Recent Developments in Two-Dimensional Carbon-Based Nanomaterials for Electrochemical Water Oxidation: A Mini Review.

Water splitting is considered a renewable and eco−friendly technique for future clean energy requirements to realize green hydrogen production, which is, to a large extent, hindered by the oxygen evolution reaction (OER) process. In recent years, two−dimensional (2D) carbon−based electrocatalysts have drawn sustained attention owing to their good electrical conductivity, unique physicochemical properties, and excellent electrocatalytic performance. Particularly, it is easy for 2D carbon−based materials to form nanocomposites, which further provides an effective strategy for electrocatalytic applications. In this review, we discuss recent advances in synthetic methods, structure−property relationships, and a basic understanding of electrocatalytic mechanisms of 2D carbon−based electrocatalysts for water oxidation. In detail, precious, non−precious metal−doped, and non−metallic 2D carbon−based electrocatalysts, as well as 2D carbon−based confined electrocatalysts, are introduced to conduct OER. Finally, current challenges, opportunities, and perspectives for further research directions of 2D carbon−based nanomaterials are outlined. This review can provide significant comprehension of high−performance 2D carbon−based electrocatalysts for water-splitting applications. [ABSTRACT FROM AUTHOR]