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Direct Copper-Free Domino Conjugate Addition-Cycloallylation using Organozinc Reagents.

Authors :
Komanduri V
Pedraza F
Krische MJ
Source :
Advanced synthesis & catalysis [Adv Synth Catal] 2008 Jul 07; Vol. 350 (10), pp. 1569-1576.
Publication Year :
2008

Abstract

The Direct Approach: Enones possessing appendant allylic carbonates react directly with diorganozinc reagents in the presence of zinc diiodide [ZnI(2)] to provide 5- and 6-membered ring products of tandem or domino conjugate addition-cycloallylation in good to excellent yield. In a related copper-free transformation, allylic carbonates are found to engage in direct allylic substitution with diorganozinc reagents.

Details

Language :
English
ISSN :
1615-4150
Volume :
350
Issue :
10
Database :
MEDLINE
Journal :
Advanced synthesis & catalysis
Publication Type :
Academic Journal
Accession number :
20454546
Full Text :
https://doi.org/10.1002/adsc.200800242