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Crystal structures, EPR and magnetic properties of 2-ClC6H4CNSSN˙ and 2,5-Cl2C6H3CNSSN˙.

Authors :
Alberola A
Carter E
Constantinides CP
Eisler DJ
Murphy DM
Rawson JM
Source :
Chemical communications (Cambridge, England) [Chem Commun (Camb)] 2011 Mar 07; Vol. 47 (9), pp. 2532-4. Date of Electronic Publication: 2011 Jan 12.
Publication Year :
2011

Abstract

The β-sheet structure associated with chlorinated aromatics (d(Cl···Cl)≈ 4.0 Å) has been implemented to drive formation of π-stacked structures of dithiadiazolyl radicals. Both title compounds exhibit an increase in paramagnetism above 150 K but solid-state EPR studies indicate that the origin of the paramagnetism in these two systems is different.

Details

Language :
English
ISSN :
1364-548X
Volume :
47
Issue :
9
Database :
MEDLINE
Journal :
Chemical communications (Cambridge, England)
Publication Type :
Academic Journal
Accession number :
21229137
Full Text :
https://doi.org/10.1039/c0cc04296j