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Evidence for a glassy state in strongly driven carbon.

Authors :
Brown CR
Gericke DO
Cammarata M
Cho BI
Döppner T
Engelhorn K
Förster E
Fortmann C
Fritz D
Galtier E
Glenzer SH
Harmand M
Heimann P
Kugland NL
Lamb DQ
Lee HJ
Lee RW
Lemke H
Makita M
Moinard A
Murphy CD
Nagler B
Neumayer P
Plagemann KU
Redmer R
Riley D
Rosmej FB
Sperling P
Toleikis S
Vinko SM
Vorberger J
White S
White TG
Wünsch K
Zastrau U
Zhu D
Tschentscher T
Gregori G
Source :
Scientific reports [Sci Rep] 2014 Jun 09; Vol. 4, pp. 5214. Date of Electronic Publication: 2014 Jun 09.
Publication Year :
2014

Abstract

Here, we report results of an experiment creating a transient, highly correlated carbon state using a combination of optical and x-ray lasers. Scattered x-rays reveal a highly ordered state with an electrostatic energy significantly exceeding the thermal energy of the ions. Strong Coulomb forces are predicted to induce nucleation into a crystalline ion structure within a few picoseconds. However, we observe no evidence of such phase transition after several tens of picoseconds but strong indications for an over-correlated fluid state. The experiment suggests a much slower nucleation and points to an intermediate glassy state where the ions are frozen close to their original positions in the fluid.

Details

Language :
English
ISSN :
2045-2322
Volume :
4
Database :
MEDLINE
Journal :
Scientific reports
Publication Type :
Academic Journal
Accession number :
24909903
Full Text :
https://doi.org/10.1038/srep05214