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Eosin Y (EY) Photoredox-Catalyzed Sulfonylation of Alkenes: Scope and Mechanism.

Authors :
Meyer AU
Straková K
Slanina T
König B
Source :
Chemistry (Weinheim an der Bergstrasse, Germany) [Chemistry] 2016 Jun 13; Vol. 22 (25), pp. 8694-9. Date of Electronic Publication: 2016 May 11.
Publication Year :
2016

Abstract

Alkyl- and aryl vinyl sulfones were obtained by eosin Y (EY)-mediated visible-light photooxidation of sulfinate salts and the reaction of the resulting S-centered radicals with alkenes. Optimized reaction conditions, the sulfinate and alkene scope, and X-ray structural analyses of several reaction products are provided. A detailed spectroscopic study explains the reaction mechanism, which proceeds through the EY radical cation as key intermediate oxidizing the sulfinate salts.<br /> (© 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.)

Details

Language :
English
ISSN :
1521-3765
Volume :
22
Issue :
25
Database :
MEDLINE
Journal :
Chemistry (Weinheim an der Bergstrasse, Germany)
Publication Type :
Academic Journal
Accession number :
27167454
Full Text :
https://doi.org/10.1002/chem.201601000