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N,B-Bidentate Boryl Ligand-Supported Iridium Catalyst for Efficient Functional-Group-Directed C-H Borylation.

Authors :
Wang G
Liu L
Wang H
Ding YS
Zhou J
Mao S
Li P
Source :
Journal of the American Chemical Society [J Am Chem Soc] 2017 Jan 11; Vol. 139 (1), pp. 91-94. Date of Electronic Publication: 2016 Dec 21.
Publication Year :
2017

Abstract

Convenient silylborane precursors for introducing N,B-bidentate boryl ligands onto transition metals were designed, prepared, and employed in ready formation of irdium(III) complexes via Si-B oxidative addition. A practical, efficient catalytic ortho-borylation reaction of arenes with a broad range of directing groups was developed using an in situ generated catalyst from the silylborane preligand 3c and [IrCl(COD)] <subscript>2</subscript> .

Details

Language :
English
ISSN :
1520-5126
Volume :
139
Issue :
1
Database :
MEDLINE
Journal :
Journal of the American Chemical Society
Publication Type :
Academic Journal
Accession number :
27992177
Full Text :
https://doi.org/10.1021/jacs.6b11867