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Doping Evolution of Magnetic Order and Magnetic Excitations in (Sr_{1-x}La_{x})_{3}Ir_{2}O_{7}.

Authors :
Lu X
McNally DE
Moretti Sala M
Terzic J
Upton MH
Casa D
Ingold G
Cao G
Schmitt T
Source :
Physical review letters [Phys Rev Lett] 2017 Jan 13; Vol. 118 (2), pp. 027202. Date of Electronic Publication: 2017 Jan 12.
Publication Year :
2017

Abstract

We use resonant elastic and inelastic x-ray scattering at the Ir-L_{3} edge to study the doping-dependent magnetic order, magnetic excitations, and spin-orbit excitons in the electron-doped bilayer iridate (Sr_{1-x}La_{x})_{3}Ir_{2}O_{7} (0≤x≤0.065). With increasing doping x, the three-dimensional long range antiferromagnetic order is gradually suppressed and evolves into a three-dimensional short range order across the insulator-to-metal transition from x=0 to 0.05, followed by a transition to two-dimensional short range order between x=0.05 and 0.065. Because of the interactions between the J_{eff}=1/2 pseudospins and the emergent itinerant electrons, magnetic excitations undergo damping, anisotropic softening, and gap collapse, accompanied by weakly doping-dependent spin-orbit excitons. Therefore, we conclude that electron doping suppresses the magnetic anisotropy and interlayer couplings and drives (Sr_{1-x}La_{x})_{3}Ir_{2}O_{7} into a correlated metallic state with two-dimensional short range antiferromagnetic order. Strong antiferromagnetic fluctuations of the J_{eff}=1/2 moments persist deep in this correlated metallic state, with the magnon gap strongly suppressed.

Details

Language :
English
ISSN :
1079-7114
Volume :
118
Issue :
2
Database :
MEDLINE
Journal :
Physical review letters
Publication Type :
Academic Journal
Accession number :
28128620
Full Text :
https://doi.org/10.1103/PhysRevLett.118.027202