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From helix to helical pores: solid-state crystalline conversions triggered by gas-solid reactions.

Authors :
Liu J
Du JJ
Wu Y
Zhao YF
Zhou XP
Li D
Source :
Chemical communications (Cambridge, England) [Chem Commun (Camb)] 2017 Nov 30; Vol. 53 (96), pp. 12950-12953.
Publication Year :
2017

Abstract

Two one-dimensional (1D) helical coordination polymers, CuBIm-Cl and CuBIm-Br (BIm = 1,2-bis((5H-imidazol-4-yl)-methylene)hydrazine), are constructed from Cu <superscript>2+</superscript> ions, halides and mono-deprotonated BIm. Solid-state crystalline conversions of CuBIm-Cl and CuBIm-Br to a gyroidal metal-organic framework (MOF) STU-3 which is composed of Cu ions and Bim ligands are observed through a gas-solid reaction, where the gas is methylamine.

Details

Language :
English
ISSN :
1364-548X
Volume :
53
Issue :
96
Database :
MEDLINE
Journal :
Chemical communications (Cambridge, England)
Publication Type :
Academic Journal
Accession number :
29159362
Full Text :
https://doi.org/10.1039/c7cc07510c