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Isolation of Cyclic(Alkyl)(Amino) Carbene-Bismuthinidene Mediated by a Beryllium(0) Complex.

Authors :
Wang G
Freeman LA
Dickie DA
Mokrai R
Benkő Z
Gilliard RJ Jr
Source :
Chemistry (Weinheim an der Bergstrasse, Germany) [Chemistry] 2019 Mar 21; Vol. 25 (17), pp. 4335-4339. Date of Electronic Publication: 2019 Feb 27.
Publication Year :
2019

Abstract

The long-sought carbene-bismuthinidene, (CAAC)Bi(Ph), has been synthesized. Notably, this represents both the first example of a carbene-stabilized subvalent bismuth complex and the extension of the carbene-pnictinidene concept to a non-toxic metallic element (Bi). The bonding has been investigated by single-crystal X-ray diffraction studies and DFT calculations. This report also highlights the hitherto unknown reducing and ligand transfer capability of a beryllium(0) complex.<br /> (© 2019 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA.)

Details

Language :
English
ISSN :
1521-3765
Volume :
25
Issue :
17
Database :
MEDLINE
Journal :
Chemistry (Weinheim an der Bergstrasse, Germany)
Publication Type :
Academic Journal
Accession number :
30706565
Full Text :
https://doi.org/10.1002/chem.201900458