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Chemoselective Synthesis of Sulfenylated Spiroindolenines from Indolyl-ynones via Organosulfenyl Chloride-Mediated Dearomatizing Spirocyclization.

Authors :
Zhang B
Li X
Ai Z
Zhao B
Yu Z
Du Y
Source :
Organic letters [Org Lett] 2022 Jan 14; Vol. 24 (1), pp. 390-394. Date of Electronic Publication: 2021 Dec 29.
Publication Year :
2022

Abstract

A metal-free sulfenylation/spirocyclization of indolyl-ynones realized by organosulfenyl chloride, generated in situ from the reaction of disulfides and PhICl <subscript>2</subscript> , is presented. This cascade one-pot process enables a chemoselective synthesis of diverse sulfenylated spiroindolenines depending on the substituent pattern at the two-position of indolyl-ynones.

Details

Language :
English
ISSN :
1523-7052
Volume :
24
Issue :
1
Database :
MEDLINE
Journal :
Organic letters
Publication Type :
Academic Journal
Accession number :
34964636
Full Text :
https://doi.org/10.1021/acs.orglett.1c04063