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Interface-Induced Conservation of Momentum Leads to Chiral-Induced Spin Selectivity.

Authors :
Vittmann C
Kessing RK
Lim J
Huelga SF
Plenio MB
Source :
The journal of physical chemistry letters [J Phys Chem Lett] 2022 Feb 24; Vol. 13 (7), pp. 1791-1796. Date of Electronic Publication: 2022 Feb 16.
Publication Year :
2022

Abstract

We study the nonequilibrium dynamics of electron transmission from a straight waveguide to a helix with spin-orbit coupling. Transmission is found to be spin-selective and can lead to large spin polarizations of the itinerant electrons. The degree of spin selectivity depends on the width of the interface region, and no polarization is found for single-point couplings. We show that this is due to momentum conservation conditions arising from extended interfaces. We therefore identify interface structure and conservation of momentum as crucial ingredients for chiral-induced spin selectivity, and we confirm that this mechanism is robust against static disorder.

Details

Language :
English
ISSN :
1948-7185
Volume :
13
Issue :
7
Database :
MEDLINE
Journal :
The journal of physical chemistry letters
Publication Type :
Academic Journal
Accession number :
35170964
Full Text :
https://doi.org/10.1021/acs.jpclett.1c03975