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Local Dynamical Heterogeneity in Simple Glass Formers.

Authors :
Biroli G
Charbonneau P
Folena G
Hu Y
Zamponi F
Source :
Physical review letters [Phys Rev Lett] 2022 Apr 29; Vol. 128 (17), pp. 175501.
Publication Year :
2022

Abstract

We study the local dynamical fluctuations in glass-forming models of particles embedded in d-dimensional space, in the mean-field limit of d→∞. Our analytical calculation reveals that single-particle observables, such as squared particle displacements, display divergent fluctuations around the dynamical (or mode-coupling) transition, due to the emergence of nontrivial correlations between displacements along different directions. This effect notably gives rise to a divergent non-Gaussian parameter, α_{2}. The d→∞ local dynamics therefore becomes quite rich upon approaching the glass transition. The finite-d remnant of this phenomenon further provides a long sought-after, first-principle explanation for the growth of α_{2} around the glass transition that is not based on multiparticle correlations.

Details

Language :
English
ISSN :
1079-7114
Volume :
128
Issue :
17
Database :
MEDLINE
Journal :
Physical review letters
Publication Type :
Academic Journal
Accession number :
35570461
Full Text :
https://doi.org/10.1103/PhysRevLett.128.175501