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Local Dynamical Heterogeneity in Simple Glass Formers.
- Source :
-
Physical review letters [Phys Rev Lett] 2022 Apr 29; Vol. 128 (17), pp. 175501. - Publication Year :
- 2022
-
Abstract
- We study the local dynamical fluctuations in glass-forming models of particles embedded in d-dimensional space, in the mean-field limit of d→∞. Our analytical calculation reveals that single-particle observables, such as squared particle displacements, display divergent fluctuations around the dynamical (or mode-coupling) transition, due to the emergence of nontrivial correlations between displacements along different directions. This effect notably gives rise to a divergent non-Gaussian parameter, α_{2}. The d→∞ local dynamics therefore becomes quite rich upon approaching the glass transition. The finite-d remnant of this phenomenon further provides a long sought-after, first-principle explanation for the growth of α_{2} around the glass transition that is not based on multiparticle correlations.
Details
- Language :
- English
- ISSN :
- 1079-7114
- Volume :
- 128
- Issue :
- 17
- Database :
- MEDLINE
- Journal :
- Physical review letters
- Publication Type :
- Academic Journal
- Accession number :
- 35570461
- Full Text :
- https://doi.org/10.1103/PhysRevLett.128.175501