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Low-dissipation self-assembly protocols of active sticky particles.

Authors :
Whitelam S
Schmit JD
Source :
Journal of crystal growth [J Cryst Growth] 2022 Dec 15; Vol. 600. Date of Electronic Publication: 2022 Oct 13.
Publication Year :
2022

Abstract

We use neuroevolutionary learning to identify time-dependent protocols for low-dissipation self-assembly in a model of generic active particles with interactions. When the time allotted for assembly is sufficiently long, low-dissipation protocols use only interparticle attractions, producing an amount of entropy that scales as the number of particles. When time is too short to allow assembly to proceed via diffusive motion, low-dissipation assembly protocols instead require particle self-propulsion, producing an amount of entropy that scales with the number of particles and the swim length required to cause assembly. Self-propulsion therefore provides an expensive but necessary mechanism for inducing assembly when time is of the essence.

Details

Language :
English
ISSN :
0022-0248
Volume :
600
Database :
MEDLINE
Journal :
Journal of crystal growth
Publication Type :
Academic Journal
Accession number :
36968622
Full Text :
https://doi.org/10.1016/j.jcrysgro.2022.126912