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Low-Temperature Heat Capacity of CsPbI 3 , Cs 4 PbI 6 , and Cs 3 Bi 2 I 9 .

Authors :
van Hattem A
Griveau JC
Colineau E
Lefering AJE
Konings RJM
Smith AL
Source :
The journal of physical chemistry. C, Nanomaterials and interfaces [J Phys Chem C Nanomater Interfaces] 2023 Nov 13; Vol. 127 (46), pp. 22808-22816. Date of Electronic Publication: 2023 Nov 13 (Print Publication: 2023).
Publication Year :
2023

Abstract

The heat capacities of CsPbI <subscript>3</subscript> , Cs <subscript>4</subscript> PbI <subscript>6</subscript> , and Cs <subscript>3</subscript> Bi <subscript>2</subscript> I <subscript>9</subscript> were studied using low-temperature thermal relaxation calorimetry in the temperature range of 1.9-300 K. The three compounds are insulators, with no electronic contribution to the heat capacity. None of them show detectable anomalies in the studied temperature window. Thermodynamic properties at standard conditions are derived. Previously reported results on Cs <subscript>3</subscript> Bi <subscript>2</subscript> I <subscript>9</subscript> are not fully consistent with the present findings. Moreover, the magnetic susceptibilities of the three title compounds were measured.<br />Competing Interests: The authors declare no competing financial interest.<br /> (© 2023 The Authors. Published by American Chemical Society.)

Details

Language :
English
ISSN :
1932-7447
Volume :
127
Issue :
46
Database :
MEDLINE
Journal :
The journal of physical chemistry. C, Nanomaterials and interfaces
Publication Type :
Academic Journal
Accession number :
38037636
Full Text :
https://doi.org/10.1021/acs.jpcc.3c05846