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Enhanced response of WO 3 thin film through Ag loading towards room temperature hydrogen gas sensor.

Authors :
T RB
Yadav PVK
Mondal A
Ramakrishnan K
Jarugala J
Liu C
Reddy YAK
Source :
Chemosphere [Chemosphere] 2024 Apr; Vol. 353, pp. 141545. Date of Electronic Publication: 2024 Feb 29.
Publication Year :
2024

Abstract

This study investigates the enhancement of hydrogen gas-sensing performance by introducing silver (Ag) nanoparticles onto tungsten trioxide (WO <subscript>3</subscript> ) thin films. Herein, the WO <subscript>3</subscript> thin films are deposited onto SiO <subscript>2</subscript> /Si substrates using a sputtering technique and Ag nanoparticles are loaded onto the WO <subscript>3</subscript> surface through a spin coating technique. To evaluate the sensing performance of a hydrogen gas, interdigitated titanium (Ti) electrodes are deposited onto the Ag:WO <subscript>3</subscript> layer. Structural, chemical, and morphological analyses are conducted for both pristine WO <subscript>3</subscript> and Ag:WO <subscript>3</subscript> thin films, followed by the investigation of gas-sensing performance by varying hydrogen gas concentrations from 100 ppm to 300 ppm and operating temperatures between 30 °C and 300 °C. The obtained results demonstrate that Ag:WO <subscript>3</subscript> thin films exhibit a notably enhanced response of 5.08% when exposed to a concentration of 100 ppm of hydrogen gas at room temperature, compared to the pristine WO <subscript>3</subscript> of 3.40%. The fabricated Ag:WO <subscript>3</subscript> sensor exhibits a response time of 3.0 s, a recovery time of 4.5 s, and also demonstrates excellent stability over 45 days period. Finally, with the superior sensitivity and fast response time, the fabricated Ti/Ag:WO <subscript>3</subscript> /Ti hydrogen gas sensor test-device can be a potential for improvement of safety from both industrial and environmental perspectives.<br />Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.<br /> (Copyright © 2024 Elsevier Ltd. All rights reserved.)

Details

Language :
English
ISSN :
1879-1298
Volume :
353
Database :
MEDLINE
Journal :
Chemosphere
Publication Type :
Academic Journal
Accession number :
38430945
Full Text :
https://doi.org/10.1016/j.chemosphere.2024.141545