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Influence of the substituents of the thiol ligand on the optical properties of AuCu 14 .

Authors :
Zhao YJ
Yang JS
Li J
Si YB
Xiao LY
Wang ZY
Hu JH
Dong XY
Zang SQ
Source :
Chemical communications (Cambridge, England) [Chem Commun (Camb)] 2024 Jul 11; Vol. 60 (57), pp. 7374-7377. Date of Electronic Publication: 2024 Jul 11.
Publication Year :
2024

Abstract

Detailed photophysical processes of two AuCu <subscript>14</subscript> clusters with different substituents (-F or -C(CH <subscript>3</subscript> ) <subscript>3</subscript> ) of the thiol ligand were studied in this work. The electronic effect of the substituents led to structural shrinkage, thus enhancing the luminous intensity. The internal conversion (IC) and intersystem crossing (ISC) rates in the AuCu14-C(CH3)3 crystal were slower compared with the AuCu14-F crystal, which was caused by the steric effect.

Details

Language :
English
ISSN :
1364-548X
Volume :
60
Issue :
57
Database :
MEDLINE
Journal :
Chemical communications (Cambridge, England)
Publication Type :
Academic Journal
Accession number :
38922126
Full Text :
https://doi.org/10.1039/d4cc01747a