Back to Search
Start Over
Broad-band lead halide perovskite quantum dot single-mode lasers.
- Source :
- Journal of Materials Chemistry C; 10/21/2020, Vol. 8 Issue 39, p13642-13647, 6p
- Publication Year :
- 2020
-
Abstract
- Perovskite colloidal quantum dots (CQDs) enable a solution-processed approach toward lasers, simultaneously providing tunable wavelength, high quantum efficiency, large absorption cross-section, and long Auger lifetimes. However, broad-band single-mode lasers based on such CQDs have been proven to be challenging. Here we report broad-band single-mode lasers from solution-processed CsPbX<subscript>3</subscript> (X = Cl, Br, I) CQDs based on a high-quality zinc oxide microrod hexagonal whispering-gallery microcavity. A typical single-mode laser with ultra-narrow linewidth (∼0.21 nm, quality factor ∼3000) at 11.7 μJ cm<superscript>−2</superscript> was obtained at 636 nm based on the conformal deposition of CsPb(Br<subscript>0.5</subscript>I<subscript>0.5</subscript>)<subscript>3</subscript> CQDs on an individual hexagonal zinc oxide microrod cavity with a radius of about ∼776 nm. Moreover, by tuning the halogen ratio, synthesis temperature and the size of the zinc oxide microrods, broad-band tunable single-mode lasers are obtained across the entire visible spectrum from 417 nm to 723 nm. These results represent a significant step towards easy solution-processed broad-band tunable single-mode lasers. [ABSTRACT FROM AUTHOR]
Details
- Language :
- English
- ISSN :
- 20507526
- Volume :
- 8
- Issue :
- 39
- Database :
- Complementary Index
- Journal :
- Journal of Materials Chemistry C
- Publication Type :
- Academic Journal
- Accession number :
- 146464801
- Full Text :
- https://doi.org/10.1039/d0tc02551h