Grid-Stretching Capability for the GEOS-Chem 13.0.0 Atmospheric Chemistry Model.

Modeling atmospheric chemistry at fine resolution globally is computationally expensive; the capability to focus on specific geographic regions using a multiscale grid is desirable. Here, we develop, validate, and demonstrate stretched-grids in the GEOS-Chem atmospheric chemistry model in its high performance implementation (GCHP). These multiscale grids are specified at runtime by four parameters that offer users nimble control of the region that is refined and the resolution of the refinement. We validate the stretched-grid simulation versus global cubed-sphere simulations. We demonstrate the operation and flexibility of stretched-grid simulations with two case studies that compare simulated tropospheric NO₂ column densities from stretched-grid and cubed-sphere simulations to retrieved column densities from the TROPOspheric Monitoring Instrument (TROPOMI). The first case study uses a stretched-grid with a broad refinement covering the contiguous US to produce simulated columns that perform similarly to a C180 (~50 km) cubed-sphere simulation at less than one-ninth the computational expense. The second case study experiments with a large stretch-factor for a global stretched-grid simulation with a highly localized refinement with ~10 km resolution for California. We find that the refinement improves spatial agreement with TROPOMI columns compared to a C90 cubed-sphere simulation of comparable computational demands, despite conducting the simulation at a finer resolution than parent meteorological fields. Overall we find that stretched-grids in GEOS-Chem are a practical tool for fine resolution regional- or continental-scale simulations of atmospheric chemistry. Stretched-grids are available in GEOS-Chem version 13.0.0. [ABSTRACT FROM AUTHOR]