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The effect of anthropogenic emission, meteorological factors, and carbon dioxide on the surface ozone increase in China from 2008 to 2018 during the East Asia summer monsoon season.

Authors :
Ma, Danyang
Wang, Tijian
Wu, Hao
Qu, Yawei
Liu, Jian
Liu, Jane
Li, Shu
Zhuang, Bingliang
Li, Mengmeng
Xie, Min
Source :
Atmospheric Chemistry & Physics; 2023, Vol. 23 Issue 11, p6525-6544, 20p
Publication Year :
2023

Abstract

Despite the implementation of the Clean Air Action Plan by the Chinese government in 2013, the issue of increasing surface ozone (O 3) concentrations remains a significant environmental concern in China. In this study, we used an improved regional climate–chemistry–ecology model (RegCM-Chem-YIBs) to investigate the impact of anthropogenic emissions, meteorological factors, and CO 2 changes on summer surface O 3 levels in China from 2008 to 2018. Compared to its predecessor, the model has been enhanced concerning the photolysis of O 3 and the radiative impacts of CO 2 and O 3. The investigations showed anthropogenic emissions were the primary contributor to the O 3 increase in China, responsible for 4.08–18.51 ppb in the North China Plain. However, changed meteorological conditions played a crucial role in decreasing O 3 in China and may have a more significant impact than anthropogenic emissions in some regions. Changed CO 2 played a critical role in the variability of O 3 through radiative forcing and isoprene emissions, particularly in southern China, inducing an increase in O 3 on the southeast coast of China (0.28–0.46 ppb) and a decrease in southwest and central China (- 0.51 to - 0.11 ppb). Our study comprehensively analyzed O 3 variation across China from various perspectives and highlighted the importance of considering CO 2 variations when designing long-term O 3 control policies, especially in high-vegetation-coverage areas. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
16807316
Volume :
23
Issue :
11
Database :
Complementary Index
Journal :
Atmospheric Chemistry & Physics
Publication Type :
Academic Journal
Accession number :
164476614
Full Text :
https://doi.org/10.5194/acp-23-6525-2023