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Electrical control of hybrid exciton transport in a van der Waals heterostructure.

Authors :
Tagarelli, Fedele
Lopriore, Edoardo
Erkensten, Daniel
Perea-Causín, Raül
Brem, Samuel
Hagel, Joakim
Sun, Zhe
Pasquale, Gabriele
Watanabe, Kenji
Taniguchi, Takashi
Malic, Ermin
Kis, Andras
Source :
Nature Photonics; Jul2023, Vol. 17 Issue 7, p615-621, 7p
Publication Year :
2023

Abstract

Interactions between out-of-plane dipoles in bosonic gases enable the long-range propagation of excitons. The lack of direct control over collective dipolar properties has so far limited the degrees of tunability and the microscopic understanding of exciton transport. In this work we modulate the layer hybridization and interplay between many-body interactions of excitons in a van der Waals heterostructure with an applied vertical electric field. By performing spatiotemporally resolved measurements supported by microscopic theory, we uncover the dipole-dependent properties and transport of excitons with different degrees of hybridization. Moreover, we find constant emission quantum yields of the transporting species as a function of excitation power with radiative decay mechanisms dominating over nonradiative ones, a fundamental requirement for efficient excitonic devices. Our findings provide a complete picture of the many-body effects in the transport of dilute exciton gases, and have crucial implications for studying emerging states of matter such as Bose–Einstein condensation and optoelectronic applications based on exciton propagation. The dipole-dependent propagation of hybrid excitons in a van der Waals heterostructure containing a WSe<subscript>2</subscript> bilayer is characterized by modulating the layer hybridization and interplay between many-body interactions of excitons with an applied vertical electric field. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
17494885
Volume :
17
Issue :
7
Database :
Complementary Index
Journal :
Nature Photonics
Publication Type :
Academic Journal
Accession number :
164720335
Full Text :
https://doi.org/10.1038/s41566-023-01198-w