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Long-lived spin waves in a metallic antiferromagnet.

Authors :
Poelchen, G.
Hellwig, J.
Peters, M.
Usachov, D. Yu.
Kliemt, K.
Laubschat, C.
Echenique, P. M.
Chulkov, E. V.
Krellner, C.
Parkin, S. S. P.
Vyalikh, D. V.
Ernst, A.
Kummer, K.
Source :
Nature Communications; 9/5/2023, Vol. 14 Issue 1, p1-8, 8p
Publication Year :
2023

Abstract

Collective spin excitations in magnetically ordered crystals, called magnons or spin waves, can serve as carriers in novel spintronic devices with ultralow energy consumption. The generation of well-detectable spin flows requires long lifetimes of high-frequency magnons. In general, the lifetime of spin waves in a metal is substantially reduced due to a strong coupling of magnons to the Stoner continuum. This makes metals unattractive for use as components for magnonic devices. Here, we present the metallic antiferromagnet CeCo<subscript>2</subscript>P<subscript>2</subscript>, which exhibits long-living magnons even in the terahertz (THz) regime. For CeCo<subscript>2</subscript>P<subscript>2</subscript>, our first-principle calculations predict a suppression of low-energy spin-flip Stoner excitations, which is verified by resonant inelastic X-ray scattering measurements. By comparison to the isostructural compound LaCo<subscript>2</subscript>P<subscript>2</subscript>, we show how small structural changes can dramatically alter the electronic structure around the Fermi level leading to the classical picture of the strongly damped magnons intrinsic to metallic systems. Our results not only demonstrate that long-lived magnons in the THz regime can exist in bulk metallic systems, but they also open a path for an efficient search for metallic magnetic systems in which undamped THz magnons can be excited. Magnons (spin-waves) in magnetic materials offer the potential for fast and efficient information processing. To avoid excessive damping due to free electrons, one is typically limited to magnetic insulators as host materials. Here, Poelchen et al demonstrate long lived spin-waves, at terahertz frequencies in the metallic antiferromaget CeCo<subscript>2</subscript>P<subscript>2</subscript>, opening up the possibility of using metallic aniferromagnets for spinwave information processing. [ABSTRACT FROM AUTHOR]

Details

Language :
English
ISSN :
20411723
Volume :
14
Issue :
1
Database :
Complementary Index
Journal :
Nature Communications
Publication Type :
Academic Journal
Accession number :
171387650
Full Text :
https://doi.org/10.1038/s41467-023-40963-x