Larger Cloud Liquid Water Enhances Both Aerosol Indirect Forcing and Cloud Radiative Feedback in Two Earth System Models.

Previous studies have noticed that the Coupled Model Intercomparison Project Phase 6 (CMIP6) models with a stronger cooling from aerosol‐cloud interactions (ACI) also have an enhanced warming from positive cloud feedback, and these two opposing effects are counter‐balanced in simulations of the historical period. However, reasons for this anti‐correlation are less explored. In this study, we perturb the cloud ice microphysical processes to obtain cloud liquid of varying amounts in two Earth System Models (ESMs). We find that the model simulations with a larger liquid water path (LWP) tend to have a stronger cooling from ACI and a stronger positive cloud feedback. More liquid clouds in the mean‐state present more opportunities for anthropogenic aerosol perturbations and also weaken the negative cloud feedback at middle to high latitudes. This work, from a cloud state perspective, emphasizes the influence of the mean‐state LWP on effective radiative forcing due to ACI (ERFACI). Plain Language Summary: Since the preindustrial era, emissions of greenhouse gases (GHGs) and aerosols have both increased substantially. Planetary warming from the elevated GHGs causes changes in cloud distribution and properties, thereby imposing feedbacks on the climate system. At the same time, aerosols from air pollution exert a cooling effect by modifying cloud properties and lifetime. Cloud feedback and aerosol‐cloud interactions (ACI) are two critical factors for understanding the past and projecting the future climate change. In this study, we examine the relationships of ACI and cloud feedback with the mean‐state cloud liquid water amount predicted from simulations with two different Earth system models. We find that both the effective radiative forcing due to aerosol‐cloud interactions (ERFACI) and the cloud feedback are modulated by mean‐state liquid water path (LWP). The warming induced by cloud feedback and cooling by ACI counteracts each other. Our study suggests that the mean‐state LWP is an important factor influencing both ERFACI and the cloud feedback, and is a useful index for the future climate projection. Key Points: Effective radiative forcing due to aerosol‐cloud interactions strengthens with the increase of mean‐state LWP in two Earth System ModelsCloud radiative feedback increases monotonically with the increase of mean‐state LWPMean‐state LWP is a good predictor for both ERFACI and cloud radiative feedback [ABSTRACT FROM AUTHOR]