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Analyzing photoionization cross-sectional modulation in CdSe/CdS core–shell nanodots: Impact of strain and applied electric field.
- Source :
- Journal of Applied Physics; 1/28/2024, Vol. 135 Issue 4, p1-9, 9p
- Publication Year :
- 2024
-
Abstract
- The role of strain in material properties is well-established, serving as a tool for altering atomic positions and defect formation, adjusting electronic structures and lattice vibrations, and influencing phase transitions, physical characteristics, and chemical properties. In this study, we conducted theoretical calculations of the binding energy and photoionization cross section (PCS) within a spherical core/shell quantum dot (CSQD) for the different transitions between the ground state of a donor impurity and the four low-lying conduction band states. During our study, we employed the finite element method to determine the energy levels and wave functions of the system within the effective mass approximation. Subsequently, we investigated the changes in PCS and binding energy while varying shell width under the influence of an applied electric field, considering both cases with and without the effect of strain. The strain effect was incorporated based on Hooke's law, and we developed specific expressions and utilized the continuum linear elasticity mechanical model for a single spherically symmetric shell. The results demonstrate that the strain correction enhances the binding energy of the four low-lying energy levels, leading to a shift of the PCS peaks toward higher energies. Conversely, the application of an external electric field has varying effects depending on the specific transition being considered. We compared our theoretical results with available experimental data and found them to be in good agreement. The pronounced blue-shift and substantial enhancement in magnitude of PCS spectra concerning shell width, electric field, and strain make CSQDs highly promising candidates for applications in adjustable nano-optoelectronic devices. [ABSTRACT FROM AUTHOR]
Details
- Language :
- English
- ISSN :
- 00218979
- Volume :
- 135
- Issue :
- 4
- Database :
- Complementary Index
- Journal :
- Journal of Applied Physics
- Publication Type :
- Academic Journal
- Accession number :
- 175161636
- Full Text :
- https://doi.org/10.1063/5.0183295