A Python tool to determine the thickness of the hydrate layer around clinker grains using SEM‐BSE images.

To accurately simulate the hydration process of cementitious materials, understanding the growth rate of C‐S‐H layers around clinker grains is crucial. Nonetheless, the thickness of the hydrate layer shows substantial variation around individual grains, depending on their surrounding. Consequently, it is not feasible to measure hydrate layers manually in a reliable and reproducible manner. To address this challenge, a software has been developed to statistically determine the C‐S‐H thickness, requiring minimal manual interventions for thresholding and for setting limits like particle size or circularity. This study presents a tool, which automatically identifies suitable clinker grains and and perform statistical measurements of their hydrate layer up to a specimen age of 28 days. The findings reveal a significant increase in the C‐S‐H layer, starting from 0.45 μm$\umu {\rm {m}}$ after 1 day and reaching 3.04 μm$\umu {\rm {m}}$ after 28 days. However, for older specimens, the measurement of the C‐S‐H layer was not feasible due to limited pore space and clinker grains. [ABSTRACT FROM AUTHOR]