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Challenges and Advances in Wide‐Temperature Electrolytes for Lithium‐Ion Batteries.
- Source :
- ChemElectroChem; 5/17/2024, Vol. 11 Issue 10, p1-19, 19p
- Publication Year :
- 2024
-
Abstract
- Lithium‐ion batteries (LIBs) have gained widespread attention due to their numerous advantages, including high energy density, prolonged cycle life, and environmental friendliness. Nevertheless, their electrochemical performance deteriorates rapidly under extreme temperature conditions, accompanied by a series of safety issues. Electrolyte optimization has emerged as a crucial and feasible strategy to expand the operational temperature range of LIBs. This review comprehensively summarizes the challenges, advances, and characterization methodologies of electrolytes at both subzero and elevated temperatures. Initially, it discusses the degradation mechanisms of different types of electrolytes at extreme temperatures, integrates recent advances, and offers insights into future research directions. Subsequently, various experimental techniques are systematically presented to evaluate the fundamental physical properties, stability, and dynamic behaviors of electrolytes in non‐ambient environments. Finally, it also provides relevant computational methods across the electronic, molecular, and macroscopic scales, and explores the application of high‐throughput techniques in this field. This review offers valuable guidance for breaking the working temperature limits of electrolytes and promoting the development of next‐generation LIBs. [ABSTRACT FROM AUTHOR]
- Subjects :
- LITHIUM-ion batteries
ELECTROLYTES
HIGH temperatures
ENERGY density
FRIENDSHIP
Subjects
Details
- Language :
- English
- ISSN :
- 21960216
- Volume :
- 11
- Issue :
- 10
- Database :
- Complementary Index
- Journal :
- ChemElectroChem
- Publication Type :
- Academic Journal
- Accession number :
- 177321265
- Full Text :
- https://doi.org/10.1002/celc.202300759