Tailoring Spin-to-Charge Conversion Efficiency via Microwave Frequency in La0.67Sr0.33MnO3/Pt Bilayer System.

The generation of spin current in materials with high spin–orbit coupling is one of the primary topics for future spintronic applications. In this context, the high conversion efficiency of spin current to charge current is desired. Ferromagnetic resonance (FMR)-based inverse spin Hall effect (ISHE) is a quite popular method to study such spin-to-charge conversion. Here microwave frequency plays a crucial role in generating spin current which further gets converted to charge current due to spin–orbit interaction of the given material. In this work, we show the effect of microwave frequency on spin-to-charge current conversion efficiency in La 0. 6 7 Sr 0. 3 3 MnO₃/Pt heterostructure prepared by oxygen-assisted molecular beam epitaxy (OMBE). From the ISHE analysis the maximum spin pumping voltage of ∼98 μV has been observed. Further spin Hall angle has been calculated for different frequencies and the maximum calculated value (∼0.06) for this system has been obtained at 14 GHz. [ABSTRACT FROM AUTHOR]