Enhanced spin–orbit torque in Pt/Sm/Co/Ta heterostructures by interface alloying with light rare-earth Sm layer.

Current-induced spin–orbit torque (SOT) has attracted much attention due to its potential applications in energy-efficient logic, memory, and artificial neuron devices. In this work, we report an enhanced SOT efficiency in perpendicularly magnetized Pt/Sm/Co/Ta heterostructures by inserting a light rare-earth Sm layer with large spin–orbit coupling. A series of Ta/Pt/Sm/Co/Ta samples with the Sm layer thickness (t_Sm) of 0, 0.6, 1.2, and 1.6 nm were prepared using direct-current magnetron sputtering. Perpendicular magnetic anisotropy, SOT efficiency, and current-driven magnetization reversal were characterized using electrical transport methods based on the anomalous Hall effect. The experimental results indicated that the switching field and magnetic anisotropic field decreased monotonically with an increase in t_Sm, while the damping-like effective field and effective spin Hall angle ( θ S H eff ) gradually increased. It demonstrates that interface modification with a Sm layer can improve the SOT efficiency and reduce the pinning potential barrier. Owing to the enhanced SOT and reduced pinning field, the critical switching current density (J_c) exhibits a steady decline when increasing t_Sm. In particular, the lowest J_c of approximately 7.83 × 10⁶ A/cm² was obtained when t_Sm was 1.6 nm. X-ray photoelectron spectroscopy revealed that electron transfer occurred between the Co, Pt, and Sm layers, which may be primarily responsible for the enhanced SOT by interface alloying to effectively strengthen the spin Hall effect of Sm and/or Pt. Our results provide a strategy for improving SOT efficiency and reducing J_c by interface alloying in SOT-based spintronic devices. [ABSTRACT FROM AUTHOR]