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Moderate-temperature thermoelectric properties of TiCoSb-based half-Heusler compounds Ti1-xTaxCoSb.
- Source :
- Journal of Applied Physics; 6/1/2007, Vol. 101 Issue 11, p113714, 6p, 2 Charts, 6 Graphs
- Publication Year :
- 2007
-
Abstract
- Ta-doped Ti<subscript>1-x</subscript>Ta<subscript>x</subscript>CoSb (0≤x≤0.08) half-Heusler compounds were synthesized by melting and annealing process. Their thermoelectric properties were studied in the temperature range of 300–900 K. The Ti<subscript>1-x</subscript>Ta<subscript>x</subscript>CoSb compounds exhibit negative Seebeck coefficients with considerably large absolute values. With increasing Ta substitution, the electrical conductivity was greatly increased, but the thermal conductivity was reduced. Because of the combined effects of increased electrical conductivity and reduced thermal conductivity, the thermoelectric performance of Ti<subscript>1-x</subscript>Ta<subscript>x</subscript>CoSb alloys was apparently improved by doping Ta. The dimensionless figure of merit of 0.3 was obtained for Ti<subscript>0.92</subscript>Ta<subscript>0.08</subscript>CoSb compound at 900 K. This value is about ten times larger than that of the undoped TiCoSb compound. [ABSTRACT FROM AUTHOR]
- Subjects :
- TANTALUM
THERMOELECTRICITY
THERMAL electromotive force
ALLOYS
MATERIALS science
Subjects
Details
- Language :
- English
- ISSN :
- 00218979
- Volume :
- 101
- Issue :
- 11
- Database :
- Complementary Index
- Journal :
- Journal of Applied Physics
- Publication Type :
- Academic Journal
- Accession number :
- 25484420
- Full Text :
- https://doi.org/10.1063/1.2738460