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CO/CO2 hydrogenation and ethylene hydroformylation over silica-supported PdZn catalysts

Authors :
Araña, J.
Homs, N.
Sales, J.
Fierro, J.L.G.
Ramirez de la Piscina, P.
Source :
Catalysis Letters; April 2001, Vol. 72 Issue: 3-4 p183-189, 7p
Publication Year :
2001

Abstract

Silica-supported PdZn catalysts have been studied in CO and CO2hydrogenation and in ethylene hydroformylation. The dilution of surface Pd by Zn lowers the hydrogenating capability of the catalysts and favours the production of higher hydrocarbons in CO hydrogenation. The catalyst with a molar ratio Pd : Zn = 3 showed an enhanced ability to insert CO into an M–alkyl bond; this catalyst produced higher oxygenates in the CO hydrogenation and was the most active in all reactions studied.

Details

Language :
English
ISSN :
1011372X and 1572879X
Volume :
72
Issue :
3-4
Database :
Supplemental Index
Journal :
Catalysis Letters
Publication Type :
Periodical
Accession number :
ejs37708861
Full Text :
https://doi.org/10.1023/A:1009053724119