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A broken translational symmetry state in an infinite-layer nickelate

Authors :
Rossi, Matteo
Osada, Motoki
Choi, Jaewon
Agrestini, Stefano
Jost, Daniel
Lee, Yonghun
Lu, Haiyu
Wang, Bai Yang
Lee, Kyuho
Nag, Abhishek
Chuang, Yi-De
Kuo, Cheng-Tai
Lee, Sang-Jun
Moritz, Brian
Devereaux, Thomas P.
Shen, Zhi-Xun
Lee, Jun-Sik
Zhou, Ke-Jin
Hwang, Harold Y.
Lee, Wei-Sheng
Source :
Nature Physics; August 2022, Vol. 18 Issue: 8 p869-873, 5p
Publication Year :
2022

Abstract

A defining signature of strongly correlated electronic systems is a rich phase diagram, which consists of multiple broken symmetries, such as magnetism, superconductivity and charge order1,2. In the recently discovered nickelate superconductors3–10, a large antiferromagnetic exchange energy has been reported, which implies the existence of strong electronic correlations11. However, signatures of a broken-symmetry state other than superconductivity have not yet been observed. Here we observe charge ordering in infinite-layer nickelates La1−xSrxNiO2using resonant X-ray scattering. The parent compound orders along the Ni–O bond direction with an incommensurate wavevector, distinct from the stripe order observed in other nickelates12–14that propagates along a direction 45° to the Ni–O bond. The resonance profile we measure indicates that ordering originates from the nickelate layers and induces a parasitic charge modulation of lanthanum electrons. Upon doping, the charge order diminishes and its wavevector shifts towards commensurate, hinting that strong electronic correlations are likely to be responsible for the ordered state. Our results suggest that the existence of charge order and its potential interplay with antiferromagnetic fluctuations and superconductivity are important themes in nickel-based superconductors.

Details

Language :
English
ISSN :
17452473 and 17452481
Volume :
18
Issue :
8
Database :
Supplemental Index
Journal :
Nature Physics
Publication Type :
Periodical
Accession number :
ejs60476958
Full Text :
https://doi.org/10.1038/s41567-022-01660-6