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Low carbon ultrasonic production of alternate fuel: Operational and mechanistic concerns of the sonochemical process of hydrogen generation under various scenarios

Authors :
Henrik Erring Hansen
Hujjatul Islam
Bruno G. Pollet
Abdulaziz Alghyamah
Kaouther Kerboua
Oualid Hamdaoui
Source :
International Journal of Hydrogen Energy. 46:26770-26787
Publication Year :
2021
Publisher :
Elsevier BV, 2021.

Abstract

Sonochemistry is considered as one of the cleaner pathways for hydrogen production. The present paper investigates the potential of this technique based upon mass, mass to energy and energy conversion metrics, using modelling and experimental approaches. Four scenarios are examined assuming four saturating gases, namely O2, air, N2 and Ar, four acoustic frequencies, i.e., 20, 210, 326 and 488 kHz, and considering common acoustic intensities then common net electric power. The study revealed that Ar is the best fitting saturating gas for the sonochemical production of hydrogen. With a common acoustic intensity of 0.48 W/cm2, an optimum ratio of H2 molar yield to acoustic energy intensity is retrieved at 210 kHz, while with a common net electric power of 87 W, the highest ratio of hydrogen yield to electric energy was observed at 20 kHz. Results were interpreted based upon emitter surface, energy conversion and distinction of calorimetric and cavitational energies.

Details

ISSN :
03603199
Volume :
46
Database :
OpenAIRE
Journal :
International Journal of Hydrogen Energy
Accession number :
edsair.doi...........46df2b8a799d15ce94f95141fdead1fa
Full Text :
https://doi.org/10.1016/j.ijhydene.2021.05.191