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Pyrocumulonimbus affect average stratospheric aerosol composition

Authors :
J. M. Katich
E. C. Apel
I. Bourgeois
C. A. Brock
T. P. Bui
P. Campuzano-Jost
R. Commane
B. Daube
M. Dollner
M. Fromm
K. D. Froyd
A. J. Hills
R. S. Hornbrook
J. L. Jimenez
A. Kupc
K. D. Lamb
K. McKain
F. Moore
D. M. Murphy
B. A. Nault
J. Peischl
A. E. Perring
D. A. Peterson
E. A. Ray
K. H. Rosenlof
T. Ryerson
G. P. Schill
J. C. Schroder
B. Weinzierl
C. Thompson
C. J. Williamson
S. C. Wofsy
P. Yu
J. P. Schwarz
Source :
Science. 379:815-820
Publication Year :
2023
Publisher :
American Association for the Advancement of Science (AAAS), 2023.

Abstract

Pyrocumulonimbus (pyroCb) are wildfire-generated convective clouds that can inject smoke directly into the stratosphere. PyroCb have been tracked for years, yet their apparent rarity and episodic nature lead to highly uncertain climate impacts. In situ measurements of pyroCb smoke reveal its distinctive and exceptionally stable aerosol properties and define the long-term influence of pyroCb activity on the stratospheric aerosol budget. Analysis of 13 years of airborne observations shows that pyroCb are responsible for 10 to 25% of the black carbon and organic aerosols in the “present-day” lower stratosphere, with similar impacts in both the North and South Hemispheres. These results suggest that, should pyroCb increase in frequency and/or magnitude in future climates, they could generate dominant trends in stratospheric aerosol.

Subjects

Subjects :
Multidisciplinary

Details

ISSN :
10959203 and 00368075
Volume :
379
Database :
OpenAIRE
Journal :
Science
Accession number :
edsair.doi...........491b566cc09cae563cda5710ec52813e
Full Text :
https://doi.org/10.1126/science.add3101