Analysis of the Magnetic Properties of RFe11Ti and RFe11TiH (R=Tb,Ho)

The values of crystalline-electric-field parameters A㎚ for RFe₁₁TiHx (R=Tb,Ho) (x=0,1) are obtained by fitting calculations to the magnetization curves along the crystal axes at 4.2 K and higher temperatures. The insertion of H element in RFe₁₁Ti significantly affects CEF parameters A㎚. By using exchange field 2μ_BHex derived by inelastic neutron scattering and fitted A㎚, the calculations reproduce the experimental curves well.