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High-performance of plasma-enhanced Zn/MCM-41 catalyst for acetylene hydration

Authors :
Bin Dai
Qinqin Wang
Sudi Zhang
Youzhu Yu
Source :
Catalysis Communications. 147:106122
Publication Year :
2020
Publisher :
Elsevier BV, 2020.

Abstract

The influence of plasma pretreatment on the catalytic performance of Zn based catalyst in acetylene hydration was studied. Furthermore, the atmosphere (N2, O2, NH3, air) and process conditions (pretreatment time, pretreatment power, gas flow) of plasma pretreatment were investigated systematically. The activity results showed that both the conversion and selectivity of the P-Zn/MCM-41 catalyst treated by oxygen plasma improved significantly. The characterization results suggested that the plasma treated catalyst enhances the mutual effect between the Zn species and MCM-41 carrier, promotes the dispersion of the active component and inhibits the loss of Zn species.

Details

ISSN :
15667367
Volume :
147
Database :
OpenAIRE
Journal :
Catalysis Communications
Accession number :
edsair.doi...........6ec16e1e3fa2ac28c8b1a9d5deb4557a
Full Text :
https://doi.org/10.1016/j.catcom.2020.106122