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Phonon sidebands of photoluminescence in single wall carbon nanotubes

Authors :
Qifeng Liang
Guili Yu
Yonglei Jia
Jinming Dong
Source :
Journal of Applied Physics. 107:024314
Publication Year :
2010
Publisher :
AIP Publishing, 2010.

Abstract

The multiphonon-assisted photoluminescence (PL) of the single wall carbon nanotubes (SWNTs) have been studied by solving the Schrodinger equation, showing a set of phonon sidebands, both the Stokes and anti-Stokes lines, which are induced by the longitudinal optical phonon and radial breathing mode phonon. All the calculated results are in a good agreement with the recent experimental PL spectra of the SWNTs [F. Plentz, H. B. Ribeiro, A. Jorio, M. S. Strano, and M. A. Pimenta, Phys. Rev. Lett. 95, 247401 (2005)] and J. Lefebvre and P. Finnie, Phys. Rev. Lett. 98, 167406 (2007)]. In addition, it is very interesting to find in the calculated PL several additional phonon sidebands with rather weak intensities, which are caused by the exciton’s coupling with two kinds of phonons, and expected to be observed in future experiments.

Details

ISSN :
10897550 and 00218979
Volume :
107
Database :
OpenAIRE
Journal :
Journal of Applied Physics
Accession number :
edsair.doi...........75ade1aa75fa1fb42968a2b81bfa9b5a