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Spinel-structure catalyst catalyzing CO2 hydrogenation to full spectrum alkenes with an ultra-high yield

Authors :
Tian-Sheng Zhao
Jinhu Wu
Rungtiwa Kosol
Lishu Shao
Guohui Yang
Noritatsu Tsubaki
Yan Zeng
Jienan Chen
Lisheng Guo
Guangbo Liu
Yu Cui
Peng Zhan
Jie Li
Source :
Chemical Communications. 56:9372-9375
Publication Year :
2020
Publisher :
Royal Society of Chemistry (RSC), 2020.

Abstract

Spinel-like ZnFe2O4 is tailor-made synthesized for catalyzing CO2 hydrogenation, achieving an ultra-high yield (1858.1 g kgcat-1 h-1) of full spectrum alkenes in a three-stage reactor system. This study provides rational design concepts from catalyst to equipment amelioration by combining promoter regulation and ex situ water removal, efficiently catalyzing CO2 into valuable chemical feedstocks with industrial potential.

Details

ISSN :
1364548X and 13597345
Volume :
56
Database :
OpenAIRE
Journal :
Chemical Communications
Accession number :
edsair.doi...........77acaf990f1608928da6958d6d4daa96
Full Text :
https://doi.org/10.1039/d0cc03426f