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Investigation of seasonal variation of compensation parameter and absorption Ångström Exponent of aerosol after loading correction over a remote station in north-east India

Authors :
Susmita Kundu
Barin Kumar De
Arup Borgohain
Rakesh Roy
Nilamoni Barman
Biswajit Saha
Anirban Guha
Source :
Atmospheric Environment. 212:106-115
Publication Year :
2019
Publisher :
Elsevier BV, 2019.

Abstract

One of the extensively used methods for aerosol mass concentration measurement is the optical filter method used in Aethalometer. Due to the aerosol loading and multi scattering effect, there are uncertainties that can lead to underestimation or overestimation of aerosol concentration and measurement of the absorption coefficient. To overcome such uncertainties, a data correction method has been adopted in the present work. During the winter, pre-monsoon and post-monsoon seasons, Aethalometer underestimated black carbon (BC) concentration by 8 ± 1%, 11 ± 1%, and 10.5 ± 0.2%, due to the higher aerosol deposition. While in the monsoon season, underestimation of 5.5 ± 2% is observed because of the presence of bigger scattering nature aerosol. For 70% of days, found a positive correlation between the compensation parameter (k880) and wavelengths, which indicated the dominance of the smaller aerosol particles. While 30% of days have a negative correlation due to the bigger aerosol particle. In the winter, pre-monsoon and monsoon seasons, the absorption coefficient at 370 nm was 86%, 90%, and 93% higher than that of 880 nm due to the higher biomass burning emissions. The absorption Angstrom exponent (α370-880) was 1.02 for fossil fuel burning and the corresponding k880 was 0.0037. In the winter and post-monsoon seasons, BC emissions from fossil fuel combustion dominated over the BC emitted by biomass burning emissions with α370-880

Details

ISSN :
13522310
Volume :
212
Database :
OpenAIRE
Journal :
Atmospheric Environment
Accession number :
edsair.doi...........79ec5a8d1409bc7749235a5032084fb7
Full Text :
https://doi.org/10.1016/j.atmosenv.2019.05.036