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Laser pulse control of photofragmentation in DCl+: The effect of carrier envelope phase

Authors :
Karl-Michael Weitzel
M. V. Korolkov
Source :
Chemical Physics. 338:277-284
Publication Year :
2007
Publisher :
Elsevier BV, 2007.

Abstract

The optically induced fragmentation of deuterium chloride ions (DCl + ) has been investigated by solving coupled time dependent Schrodinger equations. We demonstrate that the branching ratio D + :Cl + of competing reaction channels leading to either D + or Cl + can be controlled by up to a factor of 100 by means of the carrier envelope phase (CEP). This CEP effect depends on the wavelength, the intensity and on the chirp of the fs laser pulses.

Details

ISSN :
03010104
Volume :
338
Database :
OpenAIRE
Journal :
Chemical Physics
Accession number :
edsair.doi...........85e204dce8ef009e71d180ce012381d6
Full Text :
https://doi.org/10.1016/j.chemphys.2007.03.007