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Quantifying the effects of quadrupolar sinksvia15N relaxation dynamics in metronidazoles hyperpolarizedviaSABRE-SHEATH

Authors :
Eduard Y. Chekmenev
Nikita V. Chukanov
Boyd M. Goodson
Jonathan R Birchall
Igor V. Koptyug
Oleg G. Salnikov
Alexandra Svyatova
Juri G. Gelovani
Kirill V. Kovtunov
Wellington Pham
Mohammad Shah Hafez Kabir
Source :
Chemical Communications. 56:9098-9101
Publication Year :
2020
Publisher :
Royal Society of Chemistry (RSC), 2020.

Abstract

15N spin-lattice relaxation dynamics in metronidazole-15N3 and metronidazole-15N2 isotopologues are studied for rational design of 15N-enriched biomolecules for signal amplification by reversible exchange in microtesla fields. 15N relaxation dynamics mapping reveals the deleterious effects of interactions with the polarization transfer catalyst and a quadrupolar 14N nucleus within the spin-relayed 15N-15N network.

Details

ISSN :
1364548X and 13597345
Volume :
56
Database :
OpenAIRE
Journal :
Chemical Communications
Accession number :
edsair.doi...........8c41933b0bcaa1890b7b0077d8a4e9d5
Full Text :
https://doi.org/10.1039/d0cc03994b