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UV polaritons at room temperature in a microcavity containing perovskites

Authors :
Emmanuelle Deleporte
Jean-Sébastien Lauret
Xavier Lafosse
Sophie Bouchoule
Gaëtan Lanty
Source :
Journal of Luminescence. 129:1985-1988
Publication Year :
2009
Publisher :
Elsevier BV, 2009.

Abstract

The molecular crystal of ( C 6 H 5 C 2 H 4 – NH 3 ) 2 PbCl 4 perovskite presents an excitonic state with an absorption energy in the ultraviolet range (3.64 eV, 341 nm) and a large binding energy (few hundred of meV). We report here on the realization of a Perot–Fabry λ -microcavity containing a thin film of this material as active layer. Angle-resolved reflectivity and photoluminescence measurements demonstrate this microcavity works, at room temperature, in the strong coupling regime: the cavity photon mode and the excitonic state are not eigenmodes of the system any more, the new eigenmodes are a linear and coherent superposition of the exciton and photon states, called cavity polaritons.

Details

ISSN :
00222313
Volume :
129
Database :
OpenAIRE
Journal :
Journal of Luminescence
Accession number :
edsair.doi...........d2b0a0a9e2ca06aa8afc41ee2f3e33fe
Full Text :
https://doi.org/10.1016/j.jlumin.2009.04.048