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Facile Synthesis of MoS2/g-C3N4/GO Ternary Heterojunction with Enhanced Photocatalytic Activity for Water Splitting
- Source :
- ACS Sustainable Chemistry & Engineering. 5:7878-7886
- Publication Year :
- 2017
- Publisher :
- American Chemical Society (ACS), 2017.
-
Abstract
- On the basis of a simple ion exchange method, a MoS2/g-C3N4/graphene oxide (GO) ternary nanojunction was constructed as an efficient photocatalyst for hydrogen evolution using solar energy. The confinement effect in MoS2 and g-C3N4 quantum dots enhances their water-splitting redox activities. The designed heterostructure featured a band alignment that facilitates the collection of electrons in MoS2 and holes in g-C3N4, effectively suppressing the recombination of photogenerated charge carriers. Furthermore, the GO with high specific surface area serves as an excellent conductive substrate to transport holes speedily. This study thus provides a novel and facile route of establishing efficient composite photocatalyst with multinary components for energy conversion.
- Subjects :
- Materials science
General Chemical Engineering
Oxide
Nanotechnology
02 engineering and technology
010402 general chemistry
01 natural sciences
law.invention
chemistry.chemical_compound
law
Environmental Chemistry
Renewable Energy, Sustainability and the Environment
Graphene
business.industry
Heterojunction
General Chemistry
021001 nanoscience & nanotechnology
0104 chemical sciences
chemistry
Quantum dot
Photocatalysis
Water splitting
Optoelectronics
Charge carrier
0210 nano-technology
Ternary operation
business
Subjects
Details
- ISSN :
- 21680485
- Volume :
- 5
- Database :
- OpenAIRE
- Journal :
- ACS Sustainable Chemistry & Engineering
- Accession number :
- edsair.doi...........d604412af72ecd884bf2a7afc8fa6f23
- Full Text :
- https://doi.org/10.1021/acssuschemeng.7b01386