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Facile Synthesis of MoS2/g-C3N4/GO Ternary Heterojunction with Enhanced Photocatalytic Activity for Water Splitting

Authors :
Yun Zhao
Min Wang
Xiuxun Han
Peng Ju
Zhaomin Hao
Jiajia Li
Source :
ACS Sustainable Chemistry & Engineering. 5:7878-7886
Publication Year :
2017
Publisher :
American Chemical Society (ACS), 2017.

Abstract

On the basis of a simple ion exchange method, a MoS2/g-C3N4/graphene oxide (GO) ternary nanojunction was constructed as an efficient photocatalyst for hydrogen evolution using solar energy. The confinement effect in MoS2 and g-C3N4 quantum dots enhances their water-splitting redox activities. The designed heterostructure featured a band alignment that facilitates the collection of electrons in MoS2 and holes in g-C3N4, effectively suppressing the recombination of photogenerated charge carriers. Furthermore, the GO with high specific surface area serves as an excellent conductive substrate to transport holes speedily. This study thus provides a novel and facile route of establishing efficient composite photocatalyst with multinary components for energy conversion.

Details

ISSN :
21680485
Volume :
5
Database :
OpenAIRE
Journal :
ACS Sustainable Chemistry & Engineering
Accession number :
edsair.doi...........d604412af72ecd884bf2a7afc8fa6f23
Full Text :
https://doi.org/10.1021/acssuschemeng.7b01386