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Evidence for a Disordered Critical Point in a Glass-Forming Liquid

Authors :
Robert L. Jack
Ludovic Berthier
Laboratoire Charles Coulomb (L2C)
Université de Montpellier (UM)-Centre National de la Recherche Scientifique (CNRS)
University of Bath [Bath]
Source :
Physical Review Letters, Physical Review Letters, American Physical Society, 2015, 114, pp.205701. ⟨10.1103/PhysRevLett.114.205701⟩, Berthier, L & Jack, R L 2015, ' Evidence for a disordered critical point in a glass-forming liquid ', Physical Review Letters, vol. 114, no. 20, 205701, pp. 1-5 . https://doi.org/10.1103/PhysRevLett.114.205701
Publication Year :
2015
Publisher :
American Physical Society (APS), 2015.

Abstract

Using computer simulations of an atomistic glass-forming liquid, we investigate the fluctuations of the overlap between a fluid configuration and a quenched reference system. We find that large fluctuations of the overlap develop as temperature decreases, consistent with the existence of the random critical point that is predicted by effective field theories. We discuss the scaling of fluctuations near the presumed critical point, comparing the observed behaviour with that of the random-field Ising model. We argue that this critical point directly reveals the existence of an interfacial tension between amorphous metastable states, a quantity relevant both for equilibrium relaxation and for nonequilibrium melting of stable glass configurations.<br />4 figs, 5 pages

Details

ISSN :
10797114 and 00319007
Volume :
114
Database :
OpenAIRE
Journal :
Physical Review Letters
Accession number :
edsair.doi.dedup.....069f60fe0c64d834cab972b3f35a555c
Full Text :
https://doi.org/10.1103/physrevlett.114.205701