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Modulation of the activity of histone acetyltransferases by long chain alkylidenemalonates (LoCAMs)

Authors :
Ciro Milite (a)
Sabrina Castellano (a)
Rosaria Benedetti (b
Alessandra Tosco (a)
Carmen Ciliberti(a)
Caterina Vicidomini (a)
Ludovic Boully (a)
Gianluigi Franci (b
Lucia Altucci (b
Antonello Mai (e)
Gianluca Sbardella (a)
Milite, C
Castellano, S
Benedetti, R
Tosco, A
Ciliberti, C
Vicidomini, C
Boully, L
Franci, G
Altucci, Lucia
Mai, A
Sbardella, G.
Source :
Bioorganic & medicinal chemistry, 19 (2011): 3690–3701. doi:10.1016/j.bmc.2011.01.013, info:cnr-pdr/source/autori:Ciro Milite (a), Sabrina Castellano (a), Rosaria Benedetti (b, c),Alessandra Tosco (a),Carmen Ciliberti(a),Caterina Vicidomini (a),Ludovic Boully (a),Gianluigi Franci (b, d), Lucia Altucci (b, d), Antonello Mai (e), Gianluca Sbardella (a)/titolo:Modulation of the activity of histone acetyltransferases by long chain alkylidenemalonates (LoCAMs)/doi:10.1016%2Fj.bmc.2011.01.013/rivista:Bioorganic & medicinal chemistry (Print)/anno:2011/pagina_da:3690/pagina_a:3701/intervallo_pagine:3690–3701/volume:19, Bioorganic & Medicinal Chemistry
Publication Year :
2011
Publisher :
Elsevier Science Limited:Oxford Fulfillment Center, PO Box 800, Kidlington Oxford OX5 1DX United Kingdom:011 44 1865 843000, 011 44 1865 843699, EMAIL: asianfo@elsevier.com, tcb@elsevier.co.UK, INTERNET: http://www.elsevier.com, http://www.elsevier.com/locate/shpsa/, Fax: 011 44 1865 843010, 2011.

Abstract

A novel class of KAT modulators (long chain alkylidenemalonates, LoCAMs) has been identified. Variations of the alkyl chain length can change the activity profile from inhibition of both KAT3A/KAT2B (as derivative 2a) to the peculiar profile of pentadecylidenemalonate 1b, the first activator/inhibitor of histone acetyltransferases. Together with the powerful apoptotic effect (particularly notable if considering that anacardic acid and other KAT inhibitors are not cell permeable) appoint them as valuable biological tools to understand the mechanisms of lysine acetyltransferases. (C) 2011 Elsevier Ltd. All rights reserved.

Details

Language :
English
Database :
OpenAIRE
Journal :
Bioorganic & medicinal chemistry, 19 (2011): 3690–3701. doi:10.1016/j.bmc.2011.01.013, info:cnr-pdr/source/autori:Ciro Milite (a), Sabrina Castellano (a), Rosaria Benedetti (b, c),Alessandra Tosco (a),Carmen Ciliberti(a),Caterina Vicidomini (a),Ludovic Boully (a),Gianluigi Franci (b, d), Lucia Altucci (b, d), Antonello Mai (e), Gianluca Sbardella (a)/titolo:Modulation of the activity of histone acetyltransferases by long chain alkylidenemalonates (LoCAMs)/doi:10.1016%2Fj.bmc.2011.01.013/rivista:Bioorganic & medicinal chemistry (Print)/anno:2011/pagina_da:3690/pagina_a:3701/intervallo_pagine:3690–3701/volume:19, Bioorganic & Medicinal Chemistry
Accession number :
edsair.doi.dedup.....09d1f8d0acf0d1fa73d5f893653ea2e2
Full Text :
https://doi.org/10.1016/j.bmc.2011.01.013