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Width of the plasmon resonance in metal clusters

Authors :
B. Montag
P.-G. Reinhard
Source :
Physical Review B. 51:14686-14692
Publication Year :
1995
Publisher :
American Physical Society (APS), 1995.

Abstract

The width of the plasmon resonance in the clusters ${\mathrm{Na}}_{9}^{+}$, ${\mathrm{Na}}_{21}^{+}$, and ${\mathrm{Na}}_{41}^{+}$ is investigated in the framework of the structure-averaged jellium model and compared with recent experimental data. The two leading mechanisms for the line broadening are fragmentation of the resonance into nearby 1ph states and splitting through thermal quadrupole fluctuations. The fragmentation becomes activated mainly through octupole fluctuations and it gives the dominating contribution to the width.

Details

ISSN :
10953795 and 01631829
Volume :
51
Database :
OpenAIRE
Journal :
Physical Review B
Accession number :
edsair.doi.dedup.....0f5a8b1344252caa89c8cc89ca85b2a7
Full Text :
https://doi.org/10.1103/physrevb.51.14686