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Improving Charge Injection via a Blade-Coating Molybdenum Oxide Layer: Toward High-Performance Large-Area Quantum-Dot Light-Emitting Diodes
- Source :
- ACS Applied Materials & Interfaces. 10:8258-8264
- Publication Year :
- 2018
- Publisher :
- American Chemical Society (ACS), 2018.
-
Abstract
- A solution-processed molybdenum oxide (MoOx) as the hole injection layer (HIL) by doctor-blade coating was developed to improve the efficiency and lifetime of red-emitting quantum-dot light-emitting diodes (QD-LEDs). It has been demonstrated that by adding isopropyl alcohol into the MoOx precursor during the doctor-blade coating process, the morphology, composition, and the surface electronic structure of the MoOx HIL could be tailored. A high-quality MoOx film with optimized charge injection was obtained, based on which all-solution-processed highly efficient red-emitting QD-LEDs were realized by using a low-cost doctor-blade coating technique under ambient conditions. The red QD-LEDs exhibited the maximum current efficiency and external quantum efficiency of 16 cd/A and 15.1%, respectively. Moreover, the lifetime of red devices initializing at 100 cd/m2 was 3236 h under ambient conditions, which is about twice as long as those with a conventional poly(3,4-ethylenedioxythiophene)-poly(styrenesulfonate) H...
- Subjects :
- Materials science
business.industry
Isopropyl alcohol
02 engineering and technology
Electronic structure
engineering.material
010402 general chemistry
021001 nanoscience & nanotechnology
01 natural sciences
0104 chemical sciences
law.invention
chemistry.chemical_compound
Coating
chemistry
law
Quantum dot
engineering
Optoelectronics
General Materials Science
Quantum efficiency
0210 nano-technology
business
Layer (electronics)
Diode
Light-emitting diode
Subjects
Details
- ISSN :
- 19448252 and 19448244
- Volume :
- 10
- Database :
- OpenAIRE
- Journal :
- ACS Applied Materials & Interfaces
- Accession number :
- edsair.doi.dedup.....1c0dacab6ee0195961b42be4209757c9