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Nitrous oxide emissions 1999 to 2009 from a global atmospheric inversion

Authors :
Yasunori Tohjima
Shuji Aoki
Geoffrey S. Dutton
Simon O'Doherty
A. M. Crotwell
Paul B. Krummel
Takaiyo Nakazawa
L. P. Steele
Ray L. Langenfelds
Ronald G. Prinn
Ray F. Weiss
Rona Thompson
Kentaro Ishijima
Frédéric Chevallier
Paul J. Fraser
Norwegian Institute for Air Research (NILU)
Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette] (LSCE)
Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)
Modélisation INVerse pour les mesures atmosphériques et SATellitaires (SATINV)
Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)
NOAA Earth System Research Laboratory (ESRL)
National Oceanic and Atmospheric Administration (NOAA)
Commonwealth Scientific and Industrial Research Organisation [Canberra] (CSIRO)
Center for Global Change Science
Massachusetts Institute of Technology (MIT)
Scripps Institution of Oceanography (SIO - UC San Diego)
University of California [San Diego] (UC San Diego)
University of California (UC)-University of California (UC)
National Institute for Environmental Studies (NIES)
Center for Atmospheric and Oceanic Studies [Sendai]
Tohoku University [Sendai]
School of Chemistry [Bristol]
University of Bristol [Bristol]
Japan Agency for Marine-Earth Science and Technology (JAMSTEC)
Massachusetts Institute of Technology. Center for Global Change Science
Prinn, Ronald G.
Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)
Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)
Scripps Institution of Oceanography (SIO)
University of California-University of California
Source :
Atmospheric Chemistry and Physics, Atmospheric Chemistry and Physics, 2014, 14 (4), pp.1801-1817. ⟨10.5194/ACP-14-1801-2014⟩, Copernicus Publications, Atmospheric Chemistry and Physics, European Geosciences Union, 2014, 14 (4), pp.1801-1817. ⟨10.5194/ACP-14-1801-2014⟩, Atmospheric Chemistry and Physics, Vol 14, Iss 4, Pp 1801-1817 (2014)
Publication Year :
2014
Publisher :
HAL CCSD, 2014.

Abstract

N[subscript 2]O surface fluxes were estimated for 1999 to 2009 using a time-dependent Bayesian inversion technique. Observations were drawn from 5 different networks, incorporating 59 surface sites and a number of ship-based measurement series. To avoid biases in the inverted fluxes, the data were adjusted to a common scale and scale offsets were included in the optimization problem. The fluxes were calculated at the same resolution as the transport model (3.75° longitude × 2.5° latitude) and at monthly time resolution. Over the 11-year period, the global total N[subscript 2]O source varied from 17.5 to 20.1 Tg a[superscript −1] N. Tropical and subtropical land regions were found to consistently have the highest N[subscript 2]O emissions, in particular in South Asia (20 ± 3% of global total), South America (13 ± 4%) and Africa (19 ± 3%), while emissions from temperate regions were smaller: Europe (6 ± 1%) and North America (7 ± 2%). A significant multi-annual trend in N[subscript 2]O emissions (0.045 Tg a[superscript −2] N) from South Asia was found and confirms inventory estimates of this trend. Considerable interannual variability in the global N[subscript 2]O source was observed (0.8 Tg a[superscript −1] N, 1 standard deviation, SD) and was largely driven by variability in tropical and subtropical soil fluxes, in particular in South America (0.3 Tg a[superscript −1] N, 1 SD) and Africa (0.3 Tg a[superscript −1] N, 1 SD). Notable variability was also found for N[subscript 2]O fluxes in the tropical and southern oceans (0.15 and 0.2 Tg a[superscript −1] N, 1 SD, respectively). Interannual variability in the N[subscript 2]O source shows some correlation with the El Niño–Southern Oscillation (ENSO), where El Niño conditions are associated with lower N[subscript 2]O fluxes from soils and from the ocean and vice versa for La Niña conditions.

Details

Language :
English
ISSN :
16807316 and 16807324
Database :
OpenAIRE
Journal :
Atmospheric Chemistry and Physics, Atmospheric Chemistry and Physics, 2014, 14 (4), pp.1801-1817. ⟨10.5194/ACP-14-1801-2014⟩, Copernicus Publications, Atmospheric Chemistry and Physics, European Geosciences Union, 2014, 14 (4), pp.1801-1817. ⟨10.5194/ACP-14-1801-2014⟩, Atmospheric Chemistry and Physics, Vol 14, Iss 4, Pp 1801-1817 (2014)
Accession number :
edsair.doi.dedup.....2b5203ef5e091f6b5f7da090ba304389
Full Text :
https://doi.org/10.5194/ACP-14-1801-2014⟩