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Nitrous oxide emissions 1999 to 2009 from a global atmospheric inversion
- Source :
- Atmospheric Chemistry and Physics, Atmospheric Chemistry and Physics, 2014, 14 (4), pp.1801-1817. ⟨10.5194/ACP-14-1801-2014⟩, Copernicus Publications, Atmospheric Chemistry and Physics, European Geosciences Union, 2014, 14 (4), pp.1801-1817. ⟨10.5194/ACP-14-1801-2014⟩, Atmospheric Chemistry and Physics, Vol 14, Iss 4, Pp 1801-1817 (2014)
- Publication Year :
- 2014
- Publisher :
- HAL CCSD, 2014.
-
Abstract
- N[subscript 2]O surface fluxes were estimated for 1999 to 2009 using a time-dependent Bayesian inversion technique. Observations were drawn from 5 different networks, incorporating 59 surface sites and a number of ship-based measurement series. To avoid biases in the inverted fluxes, the data were adjusted to a common scale and scale offsets were included in the optimization problem. The fluxes were calculated at the same resolution as the transport model (3.75° longitude × 2.5° latitude) and at monthly time resolution. Over the 11-year period, the global total N[subscript 2]O source varied from 17.5 to 20.1 Tg a[superscript −1] N. Tropical and subtropical land regions were found to consistently have the highest N[subscript 2]O emissions, in particular in South Asia (20 ± 3% of global total), South America (13 ± 4%) and Africa (19 ± 3%), while emissions from temperate regions were smaller: Europe (6 ± 1%) and North America (7 ± 2%). A significant multi-annual trend in N[subscript 2]O emissions (0.045 Tg a[superscript −2] N) from South Asia was found and confirms inventory estimates of this trend. Considerable interannual variability in the global N[subscript 2]O source was observed (0.8 Tg a[superscript −1] N, 1 standard deviation, SD) and was largely driven by variability in tropical and subtropical soil fluxes, in particular in South America (0.3 Tg a[superscript −1] N, 1 SD) and Africa (0.3 Tg a[superscript −1] N, 1 SD). Notable variability was also found for N[subscript 2]O fluxes in the tropical and southern oceans (0.15 and 0.2 Tg a[superscript −1] N, 1 SD, respectively). Interannual variability in the N[subscript 2]O source shows some correlation with the El Niño–Southern Oscillation (ENSO), where El Niño conditions are associated with lower N[subscript 2]O fluxes from soils and from the ocean and vice versa for La Niña conditions.
- Subjects :
- [SDU.OCEAN]Sciences of the Universe [physics]/Ocean, Atmosphere
Atmospheric Science
010504 meteorology & atmospheric sciences
Climate change
Subtropics
010501 environmental sciences
01 natural sciences
lcsh:QC1-999
Latitude
lcsh:Chemistry
La Niña
lcsh:QD1-999
13. Climate action
Climatology
Soil water
Temperate climate
Environmental science
Longitude
Greenhouse effect
[SDU.ENVI]Sciences of the Universe [physics]/Continental interfaces, environment
lcsh:Physics
0105 earth and related environmental sciences
Subjects
Details
- Language :
- English
- ISSN :
- 16807316 and 16807324
- Database :
- OpenAIRE
- Journal :
- Atmospheric Chemistry and Physics, Atmospheric Chemistry and Physics, 2014, 14 (4), pp.1801-1817. ⟨10.5194/ACP-14-1801-2014⟩, Copernicus Publications, Atmospheric Chemistry and Physics, European Geosciences Union, 2014, 14 (4), pp.1801-1817. ⟨10.5194/ACP-14-1801-2014⟩, Atmospheric Chemistry and Physics, Vol 14, Iss 4, Pp 1801-1817 (2014)
- Accession number :
- edsair.doi.dedup.....2b5203ef5e091f6b5f7da090ba304389
- Full Text :
- https://doi.org/10.5194/ACP-14-1801-2014⟩