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Stroboscopic ultrafast imaging using RF strip-lines in a commercial transmission electron microscope

Authors :
Spencer A. Reisbick
Myung-Geun Han
Chuhang Liu
Yubin Zhao
Eric Montgomery
Chunguang Jing
Vikrant J. Gokhale
Jason J. Gorman
June W. Lau
Yimei Zhu
Source :
Ultramicroscopy. 235:113497
Publication Year :
2022
Publisher :
Elsevier BV, 2022.

Abstract

The development of ultrafast electron microscopy (UEM), specifically stroboscopic imaging, has brought the study of structural dynamics to a new level by overcoming the spatial limitations of ultrafast spectroscopy and the temporal restrictions of traditional TEM simultaneously. Combining the concepts governing both techniques has enabled direct visualization of dynamics with spatiotemporal resolutions in the picosecond-nanometer regime. Here, we push the limits of imaging using a pulsed electron beam via RF induced transverse deflection based on the newly developed 200 keV frequency-tunable strip-line pulser. We demonstrate a 0.2 nm spatial resolution and elucidation of magnetic spin induction maps using the phase-microscopy method. We also present beam coherence measurements and expand our study using the breathing modes of a silicon interdigitated comb under RF excitation which achieves improved temporal synchronization between the electron pulse-train and electric field. A new RF holder has also been developed with impedance matching to the RF signal to minimize transmission power loss to samples and its performance is compared with a conventional sample holder.

Details

ISSN :
03043991
Volume :
235
Database :
OpenAIRE
Journal :
Ultramicroscopy
Accession number :
edsair.doi.dedup.....492789f2e0aeec2e32b39021cb696b7a